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Stepwise isotope editing of [FeFe]-hydrogenases exposes cofactor dynamics
The six-iron cofactor of [FeFe]-hydrogenases (H-cluster) is the most efficient H(2)-forming catalyst in nature. It comprises a diiron active site with three carbon monoxide (CO) and two cyanide (CN(−)) ligands in the active oxidized state (H(ox)) and one additional CO ligand in the inhibited state (...
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| Publicado no: | Proc Natl Acad Sci U S A |
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| Main Authors: | , , , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
National Academy of Sciences
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4968730/ https://ncbi.nlm.nih.gov/pubmed/27432985 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1606178113 |
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