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Ph(i-PrO)SiH(2): An Exceptional Reductant for Metal-Catalyzed Hydrogen Atom Transfers

We report the discovery of an outstanding reductant for metal-catalyzed radical hydrofunctionalization reactions. Observations of unexpected silane solvolysis distributions in the HAT-initiated hydrogenation of alkenes reveal that phenylsilane is not the kinetically preferred reductant in many of th...

Disgrifiad llawn

Wedi'i Gadw mewn:
Manylion Llyfryddiaeth
Cyhoeddwyd yn:J Am Chem Soc
Prif Awduron: Obradors, Carla, Martinez, Ruben M., Shenvi, Ryan A.
Fformat: Artigo
Iaith:Inglês
Cyhoeddwyd: 2016
Pynciau:
Mynediad Ar-lein:https://ncbi.nlm.nih.gov/pmc/articles/PMC4858193/
https://ncbi.nlm.nih.gov/pubmed/26984323
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b02032
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