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Direct estimate of the internal π-donation to the carbene centre within N-heterocyclic carbenes and related molecules

Fifteen cyclic and acylic carbenes have been calculated with density functional theory at the BP86/def2-TZVPP level. The strength of the internal X→p(π) π-donation of heteroatoms and carbon which are bonded to the C(II) atom is estimated with the help of NBO calculations and with an energy decomposi...

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Vydáno v:Beilstein J Org Chem
Hlavní autoři: Andrada, Diego M, Holzmann, Nicole, Hamadi, Thomas, Frenking, Gernot
Médium: Artigo
Jazyk:Inglês
Vydáno: Beilstein-Institut 2015
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC4734353/
https://ncbi.nlm.nih.gov/pubmed/26877795
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.3762/bjoc.11.294
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