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Strong frequency dependence of vibrational relaxation in bulk and surface water reveals sub-picosecond structural heterogeneity
Because of strong hydrogen bonding in liquid water, intermolecular interactions between water molecules are highly delocalized. Previous two-dimensional infrared spectroscopy experiments have indicated that this delocalization smears out the structural heterogeneity of neat H(2)O. Here we report on...
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| Veröffentlicht in: | Nat Commun |
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| Hauptverfasser: | , , , , , , |
| Format: | Artigo |
| Sprache: | Inglês |
| Veröffentlicht: |
Nature Pub. Group
2015
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| Schlagworte: | |
| Online Zugang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4595750/ https://ncbi.nlm.nih.gov/pubmed/26382651 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/ncomms9384 |
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