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Highly Torquoselective Electrocyclizations and Competing 1,7-Hydrogen Shifts of 1-Azatrienes with Silyl-Substitution at the Allylic Carbon

[Image: see text] Highly torquoselective electrocyclizations of chiral 1-azatrienes are described. These 1-azatrienes contain an allylic stereocenter that is substituted with a silyl group and are derived in situ from condensation of γ-silyl-substituted enals with vinylogous amides. The ensuing ster...

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Vydáno v:Org Lett
Hlavní autoři: Ma, Zhi-Xiong, Patel, Ashay, Houk, K. N., Hsung, Richard P.
Médium: Artigo
Jazyk:Inglês
Vydáno: 2015
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On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC4547485/
https://ncbi.nlm.nih.gov/pubmed/25859907
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.5b00727
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