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10 Step Asymmetric Total Synthesis and Stereochemistry of (+)-Dragmacidin D

The asymmetric synthesis of dragmacidin D (1) has been completed in 10 steps. Its sole stereocenter was set using direct asymmetric alkylation enabled by a C(2)-symmetric tetramine and lithium N-(trimethylsilyl)-tert-butylamide as the enolization reagent. A central Larock indole synthesis was employ...

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Bibliografische gegevens
Gepubliceerd in:Angew Chem Int Ed Engl
Hoofdauteurs: Jackson, Jeffrey J., Kobayashi, Hiroyuki, Steffens, Sophia D., Zakarian, Armen
Formaat: Artigo
Taal:Inglês
Gepubliceerd in: 2015
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Online toegang:https://ncbi.nlm.nih.gov/pmc/articles/PMC4532559/
https://ncbi.nlm.nih.gov/pubmed/26130270
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201504113
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