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Functionalized Cyclopentenes Through a Tandem NHC-Catalyzed Dynamic Kinetic Resolution and Ambient Temperature Decarboxylation: Mechanistc Insight and Synthetic Application
An unusual room temperature β-lactone decarboxylation facilitated a five-step enantioselective formal synthesis of the cyclopentane core of an estrogen receptor β-agonist. A computational study probed the underlying factors facilitating unprecedented, rapid decarboxylation. Aryl substitution promote...
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| Udgivet i: | Chem Commun (Camb) |
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| Main Authors: | , , , , |
| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
2015
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4312178/ https://ncbi.nlm.nih.gov/pubmed/25575249 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c4cc09308a |
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