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Quantum delocalization of protons in the hydrogen-bond network of an enzyme active site
Enzymes use protein architectures to create highly specialized structural motifs that can greatly enhance the rates of complex chemical transformations. Here, we use experiments, combined with ab initio simulations that exactly include nuclear quantum effects, to show that a triad of strongly hydrog...
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| Publicado en: | Proc Natl Acad Sci U S A |
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| Autores principales: | , , , |
| Formato: | Artigo |
| Lenguaje: | Inglês |
| Publicado: |
National Academy of Sciences
2014
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| Materias: | |
| Acceso en línea: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4284547/ https://ncbi.nlm.nih.gov/pubmed/25503367 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1417923111 |
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