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Total synthesis of (±)-leuconolam: intramolecular allylic silane addition to a maleimide carbonyl group

A concise total synthesis of the plant alkaloid (±)-leuconolam (1) has been achieved. A regio- and diastereoselective Lewis-acid mediated allylative cyclization was used to establish, simultaneously, two adjacent tetrasubstituted carbon centers. Furthermore, an essential arene cross-coupling to a hi...

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Détails bibliographiques
Publié dans:Chem Sci
Auteurs principaux: Izgu, Enver Cagri, Hoye, Thomas R.
Format: Artigo
Langue:Inglês
Publié: 2013
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC4238231/
https://ncbi.nlm.nih.gov/pubmed/25419448
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/C3SC00056G
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