Role of pendant proton relays and proton-coupled electron transfer on the hydrogen evolution reaction by nickel hangman porphyrins

The hangman motif provides mechanistic insights into the role of pendant proton relays in governing proton-coupled electron transfer (PCET) involved in the hydrogen evolution reaction (HER). We now show improved HER activity of Ni compared with Co hangman porphyrins. Cyclic voltammogram data and sim...

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Detalhes bibliográficos
Main Authors: Bediako, D. Kwabena, Solis, Brian H., Dogutan, Dilek K., Roubelakis, Manolis M., Maher, Andrew G., Lee, Chang Hoon, Chambers, Matthew B., Hammes-Schiffer, Sharon, Nocera, Daniel G.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2014
Assuntos:
Physical Sciences
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4210285/
https://ncbi.nlm.nih.gov/pubmed/25298534
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1414908111
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