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Rhodium(III)-Catalyzed C–H Activation Mediated Synthesis of Isoquinolones from Amides and Cyclopropenes

We have developed a synthesis of 4-substituted isoquinolones from the Rh(III)-catalyzed, C–H activation mediated, coupling of O-pivaloyl benzhydroxamic acids and 3,3-disubstituted cyclopropenes. Experiments suggest the formation of a [4.1.0] bicyclic-system, which can open under acidic conditions to...

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Detalhes bibliográficos
Main Authors: Hyster, Todd K., Rovis, Tomislav
Formato: Artigo
Idioma:Inglês
Publicado em: 2013
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4206942/
https://ncbi.nlm.nih.gov/pubmed/25346576
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1055/s-0033-1339510
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