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P450-catalyzed asymmetric cyclopropanation of electron-deficient olefins under aerobic conditions

A variant of P450 from Bacillus megaterium five mutations away from wild type is a highly active catalyst for cyclopropanation of a variety of acrylamide and acrylate olefins with ethyl diazoacetate (EDA). The very high rate of reaction enabled by histidine ligation allowed the reaction to be conduc...

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Detalhes bibliográficos
Main Authors: Renata, Hans, Wang, Z. Jane, Kitto, Rebekah Z., Arnold, Frances H.
Formato: Artigo
Idioma:Inglês
Publicado em: 2014
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4159215/
https://ncbi.nlm.nih.gov/pubmed/25221671
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/C4CY00633J
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