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Aerobic Damage to [FeFe]-Hydrogenases: Activation Barriers for the Chemical Attachment of O(2)**

[FeFe]-hydrogenases are the best natural hydrogen-producing enzymes but their biotechnological exploitation is hampered by their extreme oxygen sensitivity. The free energy profile for the chemical attachment of O(2) to the enzyme active site was investigated by using a range-separated density funct...

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Detalhes bibliográficos
Main Authors: Kubas, Adam, De Sancho, David, Best, Robert B, Blumberger, Jochen
Formato: Artigo
Idioma:Inglês
Publicado em: WILEY-VCH Verlag 2014
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4143129/
https://ncbi.nlm.nih.gov/pubmed/24615978
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201400534
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