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Proton Transfer Induced SOMO-to-HOMO Level Switching in One-Electron Oxidized A-T and G-C Base Pairs: A Density Functional Theory Study

[Image: see text] In the present study, we show that for one-electron oxidized A-T or G-C base pairs the singly occupied molecular orbital (SOMO) is located on A or G and is lower in energy than the doubly occupied highest-occupied molecular orbital (HOMO) localized to the pyrimidines, T or C. This...

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Detalhes bibliográficos
Main Authors: Kumar, Anil, Sevilla, Michael D.
Formato: Artigo
Idioma:Inglês
Publicado em: American Chemical Society 2014
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4032191/
https://ncbi.nlm.nih.gov/pubmed/24798145
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jp5028004
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