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Cascade Cyclizations of Acyclic and Macrocyclic Alkynones: Studies toward the Synthesis of Phomactin A

A study of the reactivity and diastereoselectivity of the Lewis acid-promoted cascade cyclizations of both acyclic and macrocyclic alkynones is described. In these reactions, a β-iodoallenolate intermediate is generated via conjugate addition of iodide to an alkynone, followed by an intramolecular a...

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Détails bibliographiques
Auteurs principaux: Ciesielski, Jennifer, Gandon, Vincent, Frontier, Alison J.
Format: Artigo
Langue:Inglês
Publié: 2013
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC3791155/
https://ncbi.nlm.nih.gov/pubmed/23724905
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo4007514
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