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Coupling fast water exchange to slow molecular tumbling in Gd(3+) chelates: why faster is not always better
The influence of dynamics on solution state structure is a widely overlooked consideration in chemistry. Variations in Gd(3+) chelate hydration with changing coordination geometry and dissociative water exchange kinetics substantially impact the effectiveness (or relaxivity) of mono-hydrated Gd(3+)...
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| Main Authors: | , , , , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2013
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC3769110/ https://ncbi.nlm.nih.gov/pubmed/23841587 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ic400308a |
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