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A Three-Stage Mechanistic Model for Ammonia Borane Dehydrogenation by Shvo’s Catalyst

We propose a mechanistic model for three-stage dehydrogenation of ammonia borane (AB) catalyzed by Shvo’s cyclopentadienone-ligated ruthenium complex. We provide evidence for a plausible mechanism for catalyst deactivation, the transition from fast catalysis to slow catalysis, and relate those findi...

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Hlavní autoři: Lu, Zhiyao, Conley, Brian L., Williams, Travis J.
Médium: Artigo
Jazyk:Inglês
Vydáno: 2012
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC3546831/
https://ncbi.nlm.nih.gov/pubmed/23335832
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/om300562d
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