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The reaction mechanism of the enantioselective Tsuji allylation: inner-sphere and outer-sphere pathways, internal rearrangements, and asymmetric C–C bond formation
We use first principles quantum mechanics (density functional theory) to report a detailed reaction mechanism of the asymmetric Tsuji allylation involving prochiral nucleophiles and non-prochiral allyl fragments, which is consistent with experimental findings. The observed enantioselectivity is best...
Tallennettuna:
| Päätekijät: | , , , , , , , , , |
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| Aineistotyyppi: | Artigo |
| Kieli: | Inglês |
| Julkaistu: |
2012
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| Aiheet: | |
| Linkit: | https://ncbi.nlm.nih.gov/pmc/articles/PMC3537505/ https://ncbi.nlm.nih.gov/pubmed/23102088 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja306860n |
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