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Entropy-driven liquid–liquid separation in supercooled water

Twenty years ago Poole et al. suggested that the anomalous properties of supercooled water may be caused by a critical point that terminates a line of liquid–liquid separation of lower-density and higher-density water. Here we present a thermodynamic model based on this hypothesis, which describes a...

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Bibliografiske detaljer
Main Authors: Holten, V., Anisimov, M. A.
Format: Artigo
Sprog:Inglês
Udgivet: Nature Publishing Group 2012
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC3465811/
https://ncbi.nlm.nih.gov/pubmed/23056905
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/srep00713
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