Acidic ionic liquid/water solution as both medium and proton source for electrocatalytic H(2) evolution by [Ni(P(2)N(2))(2)](2+) complexes

The electrocatalytic reduction of protons to H(2) by [Image: see text] (where [Image: see text] in the highly acidic ionic liquid dibutylformamidium bis(trifluoromethanesulfonyl)amide shows a strong dependence on added water. A turnover frequency of 43,000–53,000 s(-1) has been measured for hydrogen...

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Autors principals: Pool, Douglas H., Stewart, Michael P., O’Hagan, Molly, Shaw, Wendy J., Roberts, John A. S., Bullock, R. Morris, DuBois, Daniel L.
Format: Artigo
Idioma:Inglês
Publicat: National Academy of Sciences 2012
Matèries:
Chemical Approaches to Artificial Photosynthesis: Solar Fuels Special Feature
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC3465405/
https://ncbi.nlm.nih.gov/pubmed/22685211
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1120208109
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