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Expanding the Limits of Isonitrile-Mediated Amidations: On the Remarkable Stereosubtleties of Macrolactam Formation from Synthetic Seco-Cyclosporins

The scope of isonitrile-mediated amide bond-forming reactions is further explored in this second-generation synthetic approach to cyclosporine (cyclosporin A). Both type I and type II amidations are utilized in this effort, allowing access to epimeric cyclosporins A and H from a single precursor by...

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Detalhes bibliográficos
Main Authors: Wu, Xiangyang, Stockdill, Jennifer L., Park, Peter K., Danishefsky, Samuel J.
Formato: Artigo
Idioma:Inglês
Publicado em: 2012
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3306727/
https://ncbi.nlm.nih.gov/pubmed/22280518
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja2103372
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