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Rigid Orthogonal bis-TEMPO Biradicals with Improved Solubility for Dynamic Nuclear Polarization

The synthesis and characterization of oxidized bis-thioketal-trispiro dinitroxide biradicals that orient the nitroxides in a rigid, approximately orthogonal geometry is reported. The biradicals show better performance as polarizing agents in dynamic nuclear polarization (DNP) NMR experiments as comp...

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Detalhes bibliográficos
Main Authors: Dane, Eric L., Corzilius, Björn, Rizzato, Egon, Stocker, Pierre, Maly, Thorsten, Smith, Albert A., Griffin, Robert G., Ouari, Olivier, Tordo, Paul, Swager, Timothy M.
Formato: Artigo
Idioma:Inglês
Publicado em: 2012
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3282990/
https://ncbi.nlm.nih.gov/pubmed/22304384
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo202349j
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