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Intramolecular [2+2] cycloaddition reactions of alkynyl ether-derived ketenes. A convenient synthesis of donor-acceptor cyclobutanes

[Image: see text] Mild thermolysis of tert-butyl alkynyl ethers furnishes aldoketenes, which undergo facile [2+2] cycloaddition reactions with pendant di- and trisubstituted alkenes. A wide variety of cis-fused cyclobutanones are produced in moderate to high diastereoselectivity and good to excellen...

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Detalhes bibliográficos
Main Authors: Tran, Vincent, Minehan, Thomas G.
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3244214/
https://ncbi.nlm.nih.gov/pubmed/22103709
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ol202989c
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