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Theoretical Study of the Mechanism of Oxoiron(IV) Formation from H(2)O(2) and a Nonheme Iron(II) Complex: O–O Cleavage Involving Proton-Coupled Electron Transfer

It has recently been shown that the nonheme oxoiron(IV) species supported by the 1,4,8,11-tetramethyl-1,4,8,11-tetraazacyclotetradecane ligand (TMC) can be generated in near-quantitative yield by reacting [Fe(II)(TMC)(OTf)(2)] with a stoichiometric amount of H(2)O(2) in CH(3)CN in the presence of 2,...

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Detalhes bibliográficos
Main Authors: Hirao, Hajime, Li, Feifei, Que, Lawrence, Morokuma, Keiji
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3136038/
https://ncbi.nlm.nih.gov/pubmed/21678930
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ic200522r
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