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Reactions of the Terminal Ni(II)–OH Group in Substitution and Electrophilic Reactions with Carbon Dioxide and Other Substrates: Structural Definition of Binding Modes in an Intramolecular Ni(II)…Fe(II) Bridged Site

A singular feature of the catalytic C-cluster of carbon monoxide dehydrogenase is a sulfide-bridged Ni⋯Fe locus where substrate is bound and transformed in the reversible reaction CO + H(2)O ⇌ CO(2) + 2H(+) + 2e(−). A similar structure has been sought in this work. Mononuclear planar Ni(II) complexe...

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Bibliografske podrobnosti
Main Authors: Huang, Deguang, Holm, R. H.
Format: Artigo
Jezik:Inglês
Izdano: 2010
Teme:
Online dostop:https://ncbi.nlm.nih.gov/pmc/articles/PMC3031429/
https://ncbi.nlm.nih.gov/pubmed/20218565
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja1003125
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