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Catalytic Enantioselective Total Syntheses of Bakkenolides I, J and S: Application of a Carbene-Catalyzed Desymmetrization

[Image: see text] A general strategy for the catalytic asymmetric syntheses of the bakkenolides is reported. The key bond-forming step involves an N-heterocyclic carbene catalyzed desymmetrization of a 1,3-diketone to form three new bonds in one step with excellent enantio– and diastereoselectivity....

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Detalhes bibliográficos
Main Authors: Phillips, Eric M., Roberts, John M., Scheidt, Karl A.
Formato: Artigo
Idioma:Inglês
Publicado em: 2010
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2884059/
https://ncbi.nlm.nih.gov/pubmed/20469924
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ol100938j
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