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S K-edge XAS as a Probe of Ligand-Metal Bond Covalency: Metal vs Ligand Oxidation in Cu and Ni Dithiolene Complexes

A combination of Cu L-edge and S K-edge X-ray absorption data and density functional theory (DFT) calculations have been correlated with (33)S EPR superhyperfine results to obtain the dipole integral (I(s)) for the S 1s→3p transition for the dithiolene ligand MNT (maleonitriledithiolate) in (TBA)(2)...

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Autors principals: Sarangi, Ritimukta, George, Serena DeBeer, Rudd, Deanne Jackson, Szilagyi, Robert K., Ribas, Xavi, Rovira, Concepció, Almeida, Manuel, Hodgson, Keith O., Hedman, Britt, Solomon, Edward I.
Format: Artigo
Idioma:Inglês
Publicat: 2007
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2880206/
https://ncbi.nlm.nih.gov/pubmed/17269767
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja0665949
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