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Synthesis of highly enantioenriched 3,4-dihydroquinolin-2-ones by 6-exo-trig radical cyclizations of axially chiral α-halo-ortho-alkenyl anilides

Radical cyclizations (Bu(3)SnH, Et(3)B/air, rt) of racemic α-halo-ortho-alkenyl anilides provide 3,4-dihydroquinolin-2-ones in high yield. Cyclizations of enantioenriched precursors occur in similarly high yields and with transfer of axial chirality to the new stereocenter of the products with excep...

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Sonraí Bibleagrafaíochta
Main Authors: Guthrie, David B., Geib, Steven J., Curran, Dennis P.
Formáid: Artigo
Teanga:Inglês
Foilsithe: 2009
Ábhair:
Rochtain Ar Líne:https://ncbi.nlm.nih.gov/pmc/articles/PMC2784126/
https://ncbi.nlm.nih.gov/pubmed/19799432
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja9066282
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