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Mechanism of Amido-Thiourea Catalyzed Enantioselective Imine Hydrocyanation: Transition State Stabilization via Multiple Non-Covalent Interactions

An experimental and computational investigation of amido-thiourea promoted imine hydrocyanation has revealed a new and unexpected mechanism of catalysis. Rather than direct activation of the imine by the thiourea, as had been proposed previously in related systems, the data are consistent with a mec...

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Autors principals: Zuend, Stephan J., Jacobsen, Eric N.
Format: Artigo
Idioma:Inglês
Publicat: 2009
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2783581/
https://ncbi.nlm.nih.gov/pubmed/19778044
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja9058958
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