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Metalated Nitriles: Stereodivergent Cation-Controlled Cyclizations1

Stereodivergent cyclizations of γ-hydroxy cyclohexanecarbonitriles are controlled simply through judicious choice of cation in the alkylmetal base. Deprotonating a series of cyclic γ-hydroxy nitriles with i-PrMgBr generates C-magnesiated nitriles that cyclize under stereoelectronic control to cis-fu...

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Bibliographic Details
Main Authors: Fleming, Fraser F., Wei, Yunjing, Liu, Wang, Zhang, Zhiyu
Format: Artigo
Language:Inglês
Published: 2008
Subjects:
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC2597827/
https://ncbi.nlm.nih.gov/pubmed/19657380
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1016/j.tet.2008.05.110
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