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Spectroscopic and Kinetic Studies of Perturbed Trinuclear Copper Clusters: The Role of Protons in Reductive Cleavage of the O-O Bond in the Multicopper Oxidase Fet3p
The multicopper oxidase Fet3p couples four 1e(−) oxidations of substrate to the 4e(−)reduction of O(2) to H(2)O. Fet3p uses four Cu atoms to accomplish this reaction: the type 1, type 2, and coupled binuclear type 3 sites. The type 2 and type 3 sites together form a trinuclear Cu cluster (TNC) which...
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| Main Authors: | , , , , |
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| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
2007
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC2556285/ https://ncbi.nlm.nih.gov/pubmed/17918838 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja073905m |
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