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Studies on the Mechanism-of-Action of Prekinamycin, a Member of the Diazoparaquinone Family of Natural Products: Evidence for both sp(2) Radical and Orthoquinonemethide Intermediates
The putative reductive activation chemistry of the diazoparaquinone antibiotics was modeled with Bu(3)Sn–H and prekinamycin dimethyl ether along with prekinamycin itself. Reaction in various combinations of aromatic solvents, with and without the nucleophile benzylmercaptan present, led to isolation...
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| Main Authors: | , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2006
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC2515591/ https://ncbi.nlm.nih.gov/pubmed/16984207 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja0642616 |
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