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Comparison of structures and energies of CH(5)(2+•) with CH(4)(+•) and their possible role in superacidic methane activation

Contrary to previous theoretical studies at the UHF/6-31G* level, the methonium radical dication CH(5)(2+) is not a C(s) symmetrical structure with a 2e—3c bond but a C(2v) symmetrical structure 1 with two 2e—3c bonds (at the UHF/6-31G**, UMP2/6-31G**, and UQCISD(T)/6-311G** levels). The C(s) symmet...

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Autors principals: Rasul, Golam, Prakash, G. K. Surya, Olah, George A.
Format: Artigo
Idioma:Inglês
Publicat: The National Academy of Sciences of the USA 1997
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC23401/
https://ncbi.nlm.nih.gov/pubmed/11038583
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