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Is strong hydrogen bonding in the transition state enough to account for the observed rate acceleration in a mutant of papain?

Nitriles are good inhibitors for the cysteine protease papain. However, a single amino acid mutation (Gln-19 → Glu-19) in the active site makes the mutant enzyme a good catalyst for nitrile hydrolysis. A theoretical approach was used to examine the differential transition state stabilization in the...

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Detalhes bibliográficos
Main Authors: Zheng, Ya-Jun, Bruice, Thomas C.
Formato: Artigo
Idioma:Inglês
Publicado em: The National Academy of Sciences of the USA 1997
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC20714/
https://ncbi.nlm.nih.gov/pubmed/9113981
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