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Reactivity-promoting criterion based on internal vibrational energy redistribution

We propose to introduce intrinsic dynamical properties as a criterion for promoting reactivity of small size noble metal reactive centers relevant for heterogeneous catalysis. To illustrate the concept, collisions between Ag(6)(−) or Au(6)(−) clusters and molecular oxygen have been investigated with...

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Detalhes bibliográficos
Main Authors: Mitrić, Roland, B̈rgel, Christian, Bonǎić-Koutecký, Vlasta
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2007
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC1965510/
https://ncbi.nlm.nih.gov/pubmed/17566104
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.0704066104
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