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Mechanistic Investigation of Cycloreversion/Cycloaddition Reactions between Zirconocene Metallacycle Complexes and Unsaturated Organic Substrates
Treatment of the diazametallacycle Cp(2)Zr(N(t-Bu)C=N(SiMe(3))N(SiMe(3))) (4a) with diphenylacetylene resulted in the formation of the azametallacyclobutene Cp(2)Zr(N(t-Bu)C(Ph)=C(Ph)) (6a) and Me(3)SiN=C=NSiMe(3) in high yield. A kinetic study using UV–vis spectroscopy was carried out on the transf...
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| Main Authors: | , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2001
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC1467575/ https://ncbi.nlm.nih.gov/pubmed/16724160 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/om010091o |
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