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Identification of a Pyrrole Intermediate Which Undergoes C-Glycosidation and Autoxidation to Yield the Final Product in Showdomycin Biosynthesis

Showdomycin is a C-nucleoside bearing an electrophilic maleimide base. Herein, the biosynthetic pathway of showdomycin is presented. The initial stages of the pathway involve non-ribosomal peptide synthetase (NRPS) mediated assembly of a 2-amino-1H-pyrrole-5-carboxylic acid intermediate. This interm...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Ren, Daan, Kim, Minje, Wang, Shao-An, Liu, Hung-wen
Formato: Artigo
Idioma:Inglês
Publicado em: 2021
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC8292215/
https://ncbi.nlm.nih.gov/pubmed/34048627
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202105667
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