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Lifetime-Associated Two-Dimensional Infrared Spectroscopy Reveals the Hydrogen-Bond Structure of Supercooled Water in Soft Confinement

[Image: see text] We demonstrate a method to address the problem of spectral overlap in multidimensional vibrational spectroscopy and use it to investigate supercooled aqueous sorbitol solutions. The absence of crystallization in these solutions has been attributed to “soft” confinement of water in...

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Publié dans:J Phys Chem Lett
Auteurs principaux: Caporaletti, Federico, Bonn, Daniel, Woutersen, Sander
Format: Artigo
Langue:Inglês
Publié: American Chemical Society 2021
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC8256423/
https://ncbi.nlm.nih.gov/pubmed/34157231
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jpclett.1c01595
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