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Chemical tuning of spin clock transitions in molecular monomers based on nuclear spin-free Ni(ii)

We report the existence of a sizeable quantum tunnelling splitting between the two lowest electronic spin levels of mononuclear Ni complexes. The level anti-crossing, or magnetic “clock transition”, associated with this gap has been directly monitored by heat capacity experiments. The comparison of...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Rubín-Osanz, Marcos, Lambert, François, Shao, Feng, Rivière, Eric, Guillot, Régis, Suaud, Nicolas, Guihéry, Nathalie, Zueco, David, Barra, Anne-Laure, Mallah, Talal, Luis, Fernando
Formato: Artigo
Idioma:Inglês
Publicado em: The Royal Society of Chemistry 2021
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC8179637/
https://ncbi.nlm.nih.gov/pubmed/34168771
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/d0sc05856d
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