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Shifting the scaling relations of single-atom catalysts for facile methane activation by tuning the coordination number

We investigate oxidative methane activation on a wide range of single transition metal atom catalysts embedded on N-doped graphene derivatives using density functional theory calculations. An inverse scaling relationship between *O formation and its hydrogen affinity is observed, consistent with a p...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Choi, Changhyeok, Yoon, Sungho, Jung, Yousung
Formato: Artigo
Idioma:Inglês
Publicado em: The Royal Society of Chemistry 2021
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC8179458/
https://ncbi.nlm.nih.gov/pubmed/34163628
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/d0sc05632d
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