Hydroxy-bridged resting states of a [NiFe]-hydrogenase unraveled by cryogenic vibrational spectroscopy and DFT computations

The catalytic mechanism of [NiFe]-hydrogenases is a subject of extensive research. Apart from at least four reaction intermediates of H(2)/H(+) cycling, there are also a number of resting states, which are formed under oxidizing conditions. Although not directly involved in the catalytic cycle, the...

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Tallennettuna:
Bibliografiset tiedot
Julkaisussa:Chem Sci
Päätekijät: Caserta, Giorgio, Pelmenschikov, Vladimir, Lorent, Christian, Tadjoung Waffo, Armel F., Katz, Sagie, Lauterbach, Lars, Schoknecht, Janna, Wang, Hongxin, Yoda, Yoshitaka, Tamasaku, Kenji, Kaupp, Martin, Hildebrandt, Peter, Lenz, Oliver, Cramer, Stephen P., Zebger, Ingo
Aineistotyyppi: Artigo
Kieli:Inglês
Julkaistu: The Royal Society of Chemistry 2020
Aiheet:
Chemistry
Linkit:https://ncbi.nlm.nih.gov/pmc/articles/PMC8179317/
https://ncbi.nlm.nih.gov/pubmed/34163984
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/d0sc05022a
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