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Ultrafast X-ray scattering offers a structural view of excited-state charge transfer

Intramolecular charge transfer and the associated changes in molecular structure in N,N′-dimethylpiperazine are tracked using femtosecond gas-phase X-ray scattering. The molecules are optically excited to the 3p state at 200 nm. Following rapid relaxation to the 3s state, distinct charge-localized a...

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Veröffentlicht in:Proc Natl Acad Sci U S A
Hauptverfasser: Yong, Haiwang, Xu, Xuan, Ruddock, Jennifer M., Stankus, Brian, Carrascosa, Andrés Moreno, Zotev, Nikola, Bellshaw, Darren, Du, Wenpeng, Goff, Nathan, Chang, Yu, Boutet, Sébastien, Carbajo, Sergio, Koglin, Jason E., Liang, Mengning, Robinson, Joseph S., Kirrander, Adam, Minitti, Michael P., Weber, Peter M.
Format: Artigo
Sprache:Inglês
Veröffentlicht: National Academy of Sciences 2021
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Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC8126834/
https://ncbi.nlm.nih.gov/pubmed/33947814
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.2021714118
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