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Simulating Vibronic Spectra without Born–Oppenheimer Surfaces

[Image: see text] We show how linear vibronic spectra in molecular systems can be simulated efficiently using first-principles approaches without relying on the explicit use of multiple Born–Oppenheimer potential energy surfaces. We demonstrate and analyze the performance of mean-field and beyond-me...

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Detalles Bibliográficos
Publicado en:J Phys Chem Lett
Autores principales: Lively, Kevin, Albareda, Guillermo, Sato, Shunsuke A., Kelly, Aaron, Rubio, Angel
Formato: Artigo
Lenguaje:Inglês
Publicado: American Chemical Society 2021
Acceso en línea:https://ncbi.nlm.nih.gov/pmc/articles/PMC8020382/
https://ncbi.nlm.nih.gov/pubmed/33750137
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jpclett.1c00073
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