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α-C–H Bond Functionalization of Unprotected Alicyclic Amines: Lewis Acid Promoted Addition of Enolates to Transient Imines

Enolizable cyclic imines, obtained in situ from their corresponding lithium amides by oxidation with simple ketone oxidants, are readily alkylated with a range of enolates to provide mono- and polycyclic β-aminoketones in a single operation, including the natural product (±)-myrtine. Nitrile anions...

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Vydáno v:Org Lett
Hlavní autoři: Kim, Jae Hyun, Paul, Anirudra, Ghiviriga, Ion, Seidel, Daniel
Médium: Artigo
Jazyk:Inglês
Vydáno: 2021
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On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC7924990/
https://ncbi.nlm.nih.gov/pubmed/33464093
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.0c04024
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