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Synthetic, Mechanistic and Biological Interrogation of Ginkgo biloba Chemical Space en route to (−)-Bilobalide

Here we interrogate the structurally dense (1.63 mcbits/Å(3)) GABA(A) receptor antagonist bilobalide, intermediates en route to its synthesis and related mechanistic questions. (13)C isotope labeling identifies an unexpected bromine migration en route to an α-selective, catalytic asymmetric Reformat...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Demoret, Robert M., Baker, Meghan A., Ohtawa, Masaki, Chen, Shuming, Lam, Ching Ching, Khom, Sophia, Roberto, Marisa, Forli, Stefano, Houk, Kendall N., Shenvi, Ryan A.
Formato: Artigo
Idioma:Inglês
Publicado em: 2020
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7727090/
https://ncbi.nlm.nih.gov/pubmed/32991152
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.0c08231
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