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Quantum chemical accuracy from density functional approximations via machine learning

Kohn-Sham density functional theory (DFT) is a standard tool in most branches of chemistry, but accuracies for many molecules are limited to 2-3 kcal ⋅ mol(−1) with presently-available functionals. Ab initio methods, such as coupled-cluster, routinely produce much higher accuracy, but computational...

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Detalhes bibliográficos
Publicado no:Nat Commun
Main Authors: Bogojeski, Mihail, Vogt-Maranto, Leslie, Tuckerman, Mark E., Müller, Klaus-Robert, Burke, Kieron
Formato: Artigo
Idioma:Inglês
Publicado em: Nature Publishing Group UK 2020
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7567867/
https://ncbi.nlm.nih.gov/pubmed/33067479
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/s41467-020-19093-1
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