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Surface Charges at the CaF(2)/Water Interface Allow Very Fast Intermolecular Vibrational‐Energy Transfer

We investigate the dynamics of water in contact with solid calcium fluoride, where at low pH, localized charges can develop upon fluorite dissolution. We use 2D surface‐specific vibrational spectroscopy to quantify the heterogeneity of the interfacial water (D(2)O) molecules and provide information...

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Bibliografische gegevens
Gepubliceerd in:Angew Chem Int Ed Engl
Hoofdauteurs: Lesnicki, Dominika, Zhang, Zhen, Bonn, Mischa, Sulpizi, Marialore, Backus, Ellen H. G.
Formaat: Artigo
Taal:Inglês
Gepubliceerd in: John Wiley and Sons Inc. 2020
Onderwerpen:
Online toegang:https://ncbi.nlm.nih.gov/pmc/articles/PMC7496624/
https://ncbi.nlm.nih.gov/pubmed/32239715
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202004686
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