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Fluctuating Storage of the Active Phase in a Mn‐Na(2)WO(4)/SiO(2) Catalyst for the Oxidative Coupling of Methane

Structural dynamics of a Mn‐Na(2)WO(4)/SiO(2) catalyst were detected directly under reaction conditions during the oxidative coupling of methane via in situ XRD and operando Raman spectroscopy. A new concept of fluctuating storage and release of an active phase in heterogeneous catalysis is proposed...

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Библиографические подробности
Опубликовано в: :Angew Chem Int Ed Engl
Главные авторы: Werny, Maximilian J., Wang, Yuanqing, Girgsdies, Frank, Schlögl, Robert, Trunschke, Annette
Формат: Artigo
Язык:Inglês
Опубликовано: John Wiley and Sons Inc. 2020
Предметы:
Online-ссылка:https://ncbi.nlm.nih.gov/pmc/articles/PMC7496389/
https://ncbi.nlm.nih.gov/pubmed/32364281
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202004778
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