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Resolving the structure of the E(1) state of Mo nitrogenase through Mo and Fe K-edge EXAFS and QM/MM calculations

Biological nitrogen fixation is predominately accomplished through Mo nitrogenase, which utilizes a complex MoFe(7)S(9)C catalytic cluster to reduce N(2) to NH(3). This cluster requires the accumulation of three to four reducing equivalents prior to binding N(2); however, despite decades of research...

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Vydáno v:Chem Sci
Hlavní autoři: Van Stappen, Casey, Thorhallsson, Albert Thor, Decamps, Laure, Bjornsson, Ragnar, DeBeer, Serena
Médium: Artigo
Jazyk:Inglês
Vydáno: Royal Society of Chemistry 2019
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC6984330/
https://ncbi.nlm.nih.gov/pubmed/32055350
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc02187f
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