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Strategies for Enhancing the Rate Constant of C–H Bond Cleavage by Concerted Proton-Coupled Electron Transfer

Recently the selective C–H bond cleavage under mild conditions with weak oxidants was reported for fluorenyl-benzoates. This mechanism is based on multi-site concerted proton-coupled electron transfer (PCET) involving intermolecular electron transfer to an outer-sphere oxidant coupled to intramolecu...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Sayfutyarova, Elvira R., Lam, Yan Choi, Hammes-Schiffer, Sharon
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6927470/
https://ncbi.nlm.nih.gov/pubmed/31464122
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b06849
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